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      A better way to quantify radiation damage in materials

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      It was just a piece of junk sitting in the back of a lab at the MIT Nuclear Reactor facility, ready to be disposed of. But it became the key to demonstrating a more comprehensive way of detecting atomic-level structural damage in materials — an approach that will aid the development of new materials, and could potentially support the ongoing operation of carbon-emission-free nuclear power plants, which would help alleviate global climate change.

      A tiny titanium nut that had been removed from inside the reactor was just the kind of material needed to prove that this new technique, developed at MIT and at other institutions, provides a way to probe defects created inside materials, including those that have been exposed to radiation, with five times greater sensitivity than existing methods.

      The new approach revealed that much of the damage that takes place inside reactors is at the atomic scale, and as a result is difficult to detect using existing methods. The technique provides a way to directly measure this damage through the way it changes with temperature. And it could be used to measure samples from the currently operating fleet of nuclear reactors, potentially enabling the continued safe operation of plants far beyond their presently licensed lifetimes.

      The findings are reported today in the journal Science Advances in a paper by MIT research specialist and recent graduate Charles Hirst PhD ’22; MIT professors Michael Short, Scott Kemp, and Ju Li; and five others at the University of Helsinki, the Idaho National Laboratory, and the University of California at Irvine.

      Rather than directly observing the physical structure of a material in question, the new approach looks at the amount of energy stored within that structure. Any disruption to the orderly structure of atoms within the material, such as that caused by radiation exposure or by mechanical stresses, actually imparts excess energy to the material. By observing and quantifying that energy difference, it’s possible to calculate the total amount of damage within the material — even if that damage is in the form of atomic-scale defects that are too small to be imaged with microscopes or other detection methods.

      The principle behind this method had been worked out in detail through calculations and simulations. But it was the actual tests on that one titanium nut from the MIT nuclear reactor that provided the proof — and thus opened the door to a new way of measuring damage in materials.

      The method they used is called differential scanning calorimetry. As Hirst explains, this is similar in principle to the calorimetry experiments many students carry out in high school chemistry classes, where they measure how much energy it takes to raise the temperature of a gram of water by one degree. The system the researchers used was “fundamentally the exact same thing, measuring energetic changes. … I like to call it just a fancy furnace with a thermocouple inside.”

      The scanning part has to do with gradually raising the temperature a bit at a time and seeing how the sample responds, and the differential part refers to the fact that two identical chambers are measured at once, one empty, and one containing the sample being studied. The difference between the two reveals details of the energy of the sample, Hirst explains.

      “We raise the temperature from room temperature up to 600 degrees Celsius, at a constant rate of 50 degrees per minute,” he says. Compared to the empty vessel, “your material will naturally lag behind because you need energy to heat your material. But if there are changes in the energy inside the material, that will change the temperature. In our case, there was an energy release when the defects recombine, and then it will get a little bit of a head start on the furnace … and that’s how we are measuring the energy in our sample.”

      Hirst, who carried out the work over a five-year span as his doctoral thesis project, found that contrary to what had been believed, the irradiated material showed that there were two different mechanisms involved in the relaxation of defects in titanium at the studied temperatures, revealed by two separate peaks in calorimetry. “Instead of one process occurring, we clearly saw two, and each of them corresponds to a different reaction that’s happening in the material,” he says.

      They also found that textbook explanations of how radiation damage behaves with temperature weren’t accurate, because previous tests had mostly been carried out at extremely low temperatures and then extrapolated to the higher temperatures of real-life reactor operations. “People weren’t necessarily aware that they were extrapolating, even though they were, completely,” Hirst says.

      “The fact is that our common-knowledge basis for how radiation damage evolves is based on extremely low-temperature electron radiation,” adds Short. “It just became the accepted model, and that’s what’s taught in all the books. It took us a while to realize that our general understanding was based on a very specific condition, designed to elucidate science, but generally not applicable to conditions in which we actually want to use these materials.”

      Now, the new method can be applied “to materials plucked from existing reactors, to learn more about how they are degrading with operation,” Hirst says.

      “The single biggest thing the world can do in order to get cheap, carbon-free power is to keep current reactors on the grid. They’re already paid for, they’re working,” Short adds.  But to make that possible, “the only way we can keep them on the grid is to have more certainty that they will continue to work well.” And that’s where this new way of assessing damage comes into play.

      While most nuclear power plants have been licensed for 40 to 60 years of operation, “we’re now talking about running those same assets out to 100 years, and that depends almost fully on the materials being able to withstand the most severe accidents,” Short says. Using this new method, “we can inspect them and take them out before something unexpected happens.”

      In practice, plant operators could remove a tiny sample of material from critical areas of the reactor, and analyze it to get a more complete picture of the condition of the overall reactor. Keeping existing reactors running is “the single biggest thing we can do to keep the share of carbon-free power high,” Short stresses. “This is one way we think we can do that.”

      Sergei Dudarev, a fellow at the United Kingdom Atomic Energy Authority who was not associated with this work, says this “is likely going to be impactful, as it confirms, in a nice systematic manner, supported both by experiment and simulations, the unexpectedly significant part played by the small invisible defects in microstructural evolution of materials exposed to irradiation.”

      The process is not just limited to the study of metals, nor is it limited to damage caused by radiation, the researchers say. In principle, the method could be used to measure other kinds of defects in materials, such as those caused by stresses or shockwaves, and it could be applied to materials such as ceramics or semiconductors as well.

      In fact, Short says, metals are the most difficult materials to measure with this method, and early on other researchers kept asking why this team was focused on damage to metals. That was partly because reactor components tend to be made of metal, and also because “It’s the hardest, so, if we crack this problem, we have a tool to crack them all!”

      Measuring defects in other kinds of materials can be up to 10,000 times easier than in metals, he says. “If we can do this with metals, we can make this extremely, ubiquitously applicable.” And all of it enabled by a small piece of junk that was sitting at the back of a lab.

      The research team included Fredric Granberg and Kai Nordlund at the University of Helsinki in Finland; Boopathy Kombaiah and Scott Middlemas at Idaho National Laboratory; and Penghui Cao at the University of California at Irvine. The work was supported by the U.S. National Science Foundation, an Idaho National Laboratory research grant, and a Euratom Research and Training program grant. More

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      Fusion’s newest ambassador

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      When high school senior Tuba Balta emailed MIT Plasma Science and Fusion Center (PSFC) Director Dennis Whyte in February, she was not certain she would get a response. As part of her final semester at BASIS Charter School, in Washington, she had been searching unsuccessfully for someone to sponsor an internship in fusion energy, a topic that had recently begun to fascinate her because “it’s not figured out yet.” Time was running out if she was to include the internship as part of her senior project.

      “I never say ‘no’ to a student,” says Whyte, who felt she could provide a youthful perspective on communicating the science of fusion to the general public.

      Posters explaining the basics of fusion science were being considered for the walls of a PSFC lounge area, a space used to welcome visitors who might not know much about the center’s focus: What is fusion? What is plasma? What is magnetic confinement fusion? What is a tokamak?

      Why couldn’t Balta be tasked with coming up with text for these posters, written specifically to be understandable, even intriguing, to her peers?

      Meeting the team

      Although most of the internship would be virtual, Balta visited MIT to meet Whyte and others who would guide her progress. A tour of the center showed her the past and future of the PSFC, one lab area revealing on her left the remains of the decades-long Alcator C-Mod tokamak and on her right the testing area for new superconducting magnets crucial to SPARC, designed in collaboration with MIT spinoff Commonwealth Fusion Systems.

      With Whyte, graduate student Rachel Bielajew, and Outreach Coordinator Paul Rivenberg guiding her content and style, Balta focused on one of eight posters each week. Her school also required her to keep a weekly blog of her progress, detailing what she was learning in the process of creating the posters.

      Finding her voice

      Balta admits that she was not looking forward to this part of the school assignment. But she decided to have fun with it, adopting an enthusiastic and conversational tone, as if she were sitting with friends around a lunch table. Each week, she was able to work out what she was composing for her posters and her final project by trying it out on her friends in the blog.

      Her posts won praise from her schoolmates for their clarity, as when in Week 3 she explained the concept of turbulence as it relates to fusion research, sending her readers to their kitchen faucets to experiment with the pressure and velocity of running tap water.

      The voice she found through her blog served her well during her final presentation about fusion at a school expo for classmates, parents, and the general public.

      “Most people are intimidated by the topic, which they shouldn’t be,” says Balta. “And it just made me happy to help other people understand it.”

      Her favorite part of the internship? “Getting to talk to people whose papers I was reading and ask them questions. Because when it comes to fusion, you can’t just look it up on Google.”

      Awaiting her first year at the University of Chicago, Balta reflects on the team spirit she experienced in communicating with researchers at the PSFC.

      “I think that was one of my big takeaways,” she says, “that you have to work together. And you should, because you’re always going to be missing some piece of information; but there’s always going to be somebody else who has that piece, and we can all help each other out.” More

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      Pursuing progress at the nanoscale

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      Last fall, a team of five senior undergraduate nuclear engineering students met once a week for dinners where they took turns cooking and debated how to tackle a particularly daunting challenge set forth in their program’s capstone course, 22.033 (Nuclear Systems Design Project).

      In past semesters, students had free reign to identify any real-world problem that interested them to solve through team-driven prototyping and design. This past fall worked a little differently. The team continued the trend of tackling daunting problems, but instead got an assignment to explore a particular design challenge on MIT’s campus. Rising to the challenge, the team spent the semester seeking a feasible way to introduce a highly coveted technology at MIT.

      Housed inside a big blue dome is the MIT Nuclear Reactor Laboratory (NRL). The reactor is used to conduct a wide range of science experiments, but in recent years, there have been multiple attempts to implement an instrument at the reactor that could probe the structure of materials, molecules, and devices. With this technology, researchers could model the structure of a wide range of materials and complex liquids made of polymers or containing nanoscale inhomogeneities that differ from the larger mass. On campus, researchers for the first time could conduct experiments to better understand the properties and functions of anything placed in front of a neutron beam emanating from the reactor core.

      The impact of this would be immense. If the reactor could be adapted to conduct this advanced technique, known as small-angle neutron scattering (SANS), it would open up a whole new world of research at MIT.

      “It’s essentially using the nuclear reactor as an incredibly high-performance camera that researchers from all over MIT would be very interested in using, including nuclear science and engineering, chemical engineering, biological engineering, and materials science, who currently use this tool at other institutions,” says Zachary Hartwig, Nuclear Systems Design Project professor and the MIT Robert N. Noyce Career Development Professor.

      SANS instruments have been installed at fewer than 20 facilities worldwide, and MIT researchers have previously considered implementing the capability at the reactor to help MIT expand community-wide access to SANS. Last fall, this mission went from long-time campus dream to potential reality as it became the design challenge that Hartwig’s students confronted. Despite having no experience with SANS, the team embraced the challenge, taking the first steps to figure out how to bring this technology to campus.

      “I really loved the idea that what we were doing could have a very real impact,” says Zoe Fisher, Nuclear Systems Design Project team member and now graduate nuclear engineering student.

      Each fall, Hartwig uses the course to introduce students to real-world challenges with strict constraints on solutions, and last fall’s project came with plenty of thorny design questions for students to tackle. First was the size limitation posed by the space available at MIT’s reactor. In SANS facilities around the world, the average length of the instrument is 30 meters, but at NRL, the space available is approximately 7.5 meters. Second, these instruments can cost up to $30 million, which is far outside NRL’s proposed budget of $3 million. That meant not only did students need to design an instrument that would work in a smaller space, but also one that could be built for a tenth of the typical cost.

      “The challenge was not just implementing one of these instruments,” Hartwig says. “It was whether the students could significantly innovate beyond the ‘traditional’ approach to doing SANS to meet the daunting constraints that we have at the MIT Reactor.”

      Because NRL actually wants to pursue this project, the students had to get creative, and their creative potential was precisely why the idea arose to get them involved, says Jacopo Buongiorno, the director of science and technology at NRL and Tokyo Electric Power Company Professor in Nuclear Engineering. “Involvement in real-world projects that answer questions about feasibility and cost of new technology and capabilities is a key element of a successful undergraduate education at MIT,” Buongiorno says.

      Students say it would have been impossible to tackle the problem without the help of co-instructor Boris Khaykovich, a research scientist at NRL who specializes in neutron instrumentation.

      Over the past two decades, Khaykovich has watched as SANS became the most popular technique for analyzing material structure. As the amount of available SANS beam time at the few facilities that exist became more competitive, access declined. Today only the experiments passing the most stringent review get access. What Khaykovich hopes to bring to MIT is improved access to SANS by designing an instrument that will be suitable for a majority of run-of-the-mill experiments, even if it’s not as powerful as state-of-the-art national SANS facilities. Such an instrument can still serve a wider range of researchers who currently have few opportunities to pursue SANS experiments.

      “In the U.S., we don’t have a simple, small, day-to-day SANS instrument,” Khaykovich says.

      With Khaykovich’s help, nuclear engineering undergraduate student Liam Hines says his team was able to go much further with their assessment than they would’ve starting from scratch, with no background in SANS. This project was unlike anything they’d ever been asked of as MIT students, and for students like Hines, who contributed to NRL research his entire time on campus, it was a project that hit close to home. “We were imagining this thing that might be designed at MIT,” Hines says.

      Fisher and Hines were joined by undergraduate nuclear engineering student team members Francisco Arellano, Jovier Jimenez, and Brendan Vaughan. Together, they devised a design that surprised both Khaykovich and Hartwig, identifying creative solutions that overcame all limitations and significantly reduced cost.

      Their team’s final project featured an adaptation of a conical design that was recently experimentally tested in Japan, but not generally used. The conical design allowed them to maximize precision while working within the other constraints, resulting in an instrument design that exceeded Hartwig’s expectations. The students also showed the feasibility of using an alternative type of glass-based low-cost neutron detector to calibrate the scattering data. By avoiding the need for a traditional detector based on helium-3, which is increasingly scarce and exorbitantly expensive, such a detector would dramatically reduce cost and increase availability. Their final presentation indicated the day-to-day SANS instrument could be built at only 4.5 meters long and with an estimated cost less than $1 million.

      Khaykovich credited the students for their enthusiasm, bouncing ideas off each other and exploring as much terrain as possible by interviewing experts who implemented SANS at other facilities. “They showed quite a perseverance and an ability to go deep into a very unfamiliar territory for them,” Khaykovich says.

      Hines says that Hartwig emphasized the importance of fielding expert opinions to more quickly discover optimal solutions. Fisher says that based on their research, if their design is funded, it would make SANS “more accessible to research for the sake of knowledge,” rather than dominated by industry research.

      Hartwig and Khaykovich agreed the students’ final project results showed a baseline of how MIT could pursue SANS technology cheaply, and when NRL proceeds with its own design process, Hartwig says, “The student’s work might actually change the cost of the feasibility of this at MIT in a way that if we hadn’t run the class, we would never have thought about doing.”

      Buongiorno says as they move forward with the project, NRL staff will consult students’ findings.

      “Indeed, the students developed original technical approaches, which are now being further explored by the NRL staff and may ultimately lead to the deployment of this new important capability on the MIT campus,” Buongiorno says.

      Hartwig says it’s a goal of the Nuclear Systems Design Project course to empower students to learn how to lead teams and embrace challenges, so they can be effective leaders advancing novel solutions in research and industry. “I think it helps teach people to be agile, to be flexible, to have confidence that they can actually go off and learn what they don’t know and solve problems they may think are bigger than themselves,” he says.

      It’s common for past classes of Nuclear Systems Design Project students to continue working on ideas beyond the course, and some students have even launched companies from their project research. What’s less common is for Hartwig’s students to actively serve as engineers pointed to a particular campus problem that’s expected to be resolved in the next few years.

      “In this case, they’re actually working on something real,” Hartwig says. “Their ideas are going to very much influence what we hope will be a facility that gets built at the reactor.”

      For students, it was exciting to inform a major instrument proposal that will soon be submitted to federal funding agencies, and for Hines, it became a chance to make his mark at NRL.

      “This is a lab I’ve been contributing to my entire time at MIT, and then through this project, I finished my time at MIT contributing in a much larger sense,” Hines says. More

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      Evan Leppink: Seeking a way to better stabilize the fusion environment

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      “Fusion energy was always one of those kind-of sci-fi technologies that you read about,” says nuclear science and engineering PhD candidate Evan Leppink. He’s recalling the time before fusion became a part of his daily hands-on experience at MIT’s Plasma Science and Fusion Center, where he is studying a unique way to drive current in a tokamak plasma using radiofrequency (RF) waves. 

      Now, an award from the U.S. Department of Energy’s (DOE) Office of Science Graduate Student Research (SCGSR) Program will support his work with a 12-month residency at the DIII-D National Fusion Facility in San Diego, California.

      Like all tokamaks, DIII-D generates hot plasma inside a doughnut-shaped vacuum chamber wrapped with magnets. Because plasma will follow magnetic field lines, tokamaks are able to contain the turbulent plasma fuel as it gets hotter and denser, keeping it away from the edges of the chamber where it could damage the wall materials. A key part of the tokamak concept is that part of the magnetic field is created by electrical currents in the plasma itself, which helps to confine and stabilize the configuration. Researchers often launch high-power RF waves into tokamaks to drive that current.

      Leppink will be contributing to research, led by his MIT advisor Steve Wukitch, that pursues launching RF waves in DIII-D using a unique compact antenna placed on the tokamak center column. Typically, antennas are placed inside the tokamak on the outer edge of the doughnut, farthest from the central hole (or column), primarily because access and installation are easier there. This is known as the “low-field side,” because the magnetic field is lower there than at the central column, the “high-field side.” This MIT-led experiment, for the first time, will mount an antenna on the high-field side. There is some theoretical evidence that placing the wave launcher there could improve power penetration and current drive efficiency. And because the plasma environment is less harsh on this side, the antenna will survive longer, a factor important for any future power-producing tokamak.

      Leppink’s work on DIII-D focuses specifically on measuring the density of plasmas generated in the tokamak, for which he developed a “reflectometer.” This small antenna launches microwaves into the plasma, which reflect back to the antenna to be measured. The time that it takes for these microwaves to traverse the plasma provides information about the plasma density, allowing researchers to build up detailed density profiles, data critical for injecting RF power into the plasma.

      “Research shows that when we try to inject these waves into the plasma to drive the current, they can lose power as they travel through the edge region of the tokamak, and can even have problems entering the core of the plasma, where we would most like to direct them,” says Leppink. “My diagnostic will measure that edge region on the high-field side near the launcher in great detail, which provides us a way to directly verify calculations or compare actual results with simulation results.”

      Although focused on his own research, Leppink has excelled at priming other students for success in their studies and research. In 2021 he received the NSE Outstanding Teaching Assistant and Mentorship Award.

      “The highlights of TA’ing for me were the times when I could watch students go from struggling with a difficult topic to fully understanding it, often with just a nudge in the right direction and then allowing them to follow their own intuition the rest of the way,” he says.

      The right direction for Leppink points toward San Diego and RF current drive experiments on DIII-D. He is grateful for the support from the SCGSR, a program created to prepare graduate students like him for science, technology, engineering, or mathematics careers important to the DOE Office of Science mission. It provides graduate thesis research opportunities through extended residency at DOE national laboratories. He has already made several trips to DIII-D, in part to install his reflectometer, and has been impressed with the size of the operation.

      “It takes a little while to kind of compartmentalize everything and say, ‘OK, well, here’s my part of the machine. This is what I’m doing.’ It can definitely be overwhelming at times. But I’m blessed to be able to work on what has been the workhorse tokamak of the United States for the past few decades.” More

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      MIT expands research collaboration with Commonwealth Fusion Systems to build net energy fusion machine, SPARC

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      MIT’s Plasma Science and Fusion Center (PSFC) will substantially expand its fusion energy research and education activities under a new five-year agreement with Institute spinout Commonwealth Fusion Systems (CFS).

      “This expanded relationship puts MIT and PSFC in a prime position to be an even stronger academic leader that can help deliver the research and education needs of the burgeoning fusion energy industry, in part by utilizing the world’s first burning plasma and net energy fusion machine, SPARC,” says PSFC director Dennis Whyte. “CFS will build SPARC and develop a commercial fusion product, while MIT PSFC will focus on its core mission of cutting-edge research and education.”

      Commercial fusion energy has the potential to play a significant role in combating climate change, and there is a concurrent increase in interest from the energy sector, governments, and foundations. The new agreement, administered by the MIT Energy Initiative (MITEI), where CFS is a startup member, will help PSFC expand its fusion technology efforts with a wider variety of sponsors. The collaboration enables rapid execution at scale and technology transfer into the commercial sector as soon as possible.

      This new agreement doubles CFS’ financial commitment to PSFC, enabling greater recruitment and support of students, staff, and faculty. “We’ll significantly increase the number of graduate students and postdocs, and just as important they will be working on a more diverse set of fusion science and technology topics,” notes Whyte. It extends the collaboration between PSFC and CFS that resulted in numerous advances toward fusion power plants, including last fall’s demonstration of a high-temperature superconducting (HTS) fusion electromagnet with record-setting field strength of 20 tesla.

      The combined magnetic fusion efforts at PSFC will surpass those in place during the operations of the pioneering Alcator C-Mod tokamak device that operated from 1993 to 2016. This increase in activity reflects a moment when multiple fusion energy technologies are seeing rapidly accelerating development worldwide, and the emergence of a new fusion energy industry that would require thousands of trained people.

      MITEI director Robert Armstrong adds, “Our goal from the beginning was to create a membership model that would allow startups who have specific research challenges to leverage the MITEI ecosystem, including MIT faculty, students, and other MITEI members. The team at the PSFC and MITEI have worked seamlessly to support CFS, and we are excited for this next phase of the relationship.”

      PSFC is supporting CFS’ efforts toward realizing the SPARC fusion platform, which facilitates rapid development and refinement of elements (including HTS magnets) needed to build ARC, a compact, modular, high-field fusion power plant that would set the stage for commercial fusion energy production. The concepts originated in Whyte’s nuclear science and engineering class 22.63 (Principles of Fusion Engineering) and have been carried forward by students and PSFC staff, many of whom helped found CFS; the new activity will expand research into advanced technologies for the envisioned pilot plant.

      “This has been an incredibly effective collaboration that has resulted in a major breakthrough for commercial fusion with the successful demonstration of revolutionary fusion magnet technology that will enable the world’s first commercially relevant net energy fusion device, SPARC, currently under construction,” says Bob Mumgaard SM ’15, PhD ’15, CEO of Commonwealth Fusion Systems. “We look forward to this next phase in the collaboration with MIT as we tackle the critical research challenges ahead for the next steps toward fusion power plant development.”

      In the push for commercial fusion energy, the next five years are critical, requiring intensive work on materials longevity, heat transfer, fuel recycling, maintenance, and other crucial aspects of power plant development. It will need innovation from almost every engineering discipline. “Having great teams working now, it will cut the time needed to move from SPARC to ARC, and really unleash the creativity. And the thing MIT does so well is cut across disciplines,” says Whyte.

      “To address the climate crisis, the world needs to deploy existing clean energy solutions as widely and as quickly as possible, while at the same time developing new technologies — and our goal is that those new technologies will include fusion power,” says Maria T. Zuber, MIT’s vice president for research. “To make new climate solutions a reality, we need focused, sustained collaborations like the one between MIT and Commonwealth Fusion Systems. Delivering fusion power onto the grid is a monumental challenge, and the combined capabilities of these two organizations are what the challenge demands.”

      On a strategic level, climate change and the imperative need for widely implementable carbon-free energy have helped orient the PSFC team toward scalability. “Building one or 10 fusion plants doesn’t make a difference — we have to build thousands,” says Whyte. “The design decisions we make will impact the ability to do that down the road. The real enemy here is time, and we want to remove as many impediments as possible and commit to funding a new generation of scientific leaders. Those are critically important in a field with as much interdisciplinary integration as fusion.” More

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      Machine learning, harnessed to extreme computing, aids fusion energy development

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      MIT research scientists Pablo Rodriguez-Fernandez and Nathan Howard have just completed one of the most demanding calculations in fusion science — predicting the temperature and density profiles of a magnetically confined plasma via first-principles simulation of plasma turbulence. Solving this problem by brute force is beyond the capabilities of even the most advanced supercomputers. Instead, the researchers used an optimization methodology developed for machine learning to dramatically reduce the CPU time required while maintaining the accuracy of the solution.

      Fusion energyFusion offers the promise of unlimited, carbon-free energy through the same physical process that powers the sun and the stars. It requires heating the fuel to temperatures above 100 million degrees, well above the point where the electrons are stripped from their atoms, creating a form of matter called plasma. On Earth, researchers use strong magnetic fields to isolate and insulate the hot plasma from ordinary matter. The stronger the magnetic field, the better the quality of the insulation that it provides.

      Rodriguez-Fernandez and Howard have focused on predicting the performance expected in the SPARC device, a compact, high-magnetic-field fusion experiment, currently under construction by the MIT spin-out company Commonwealth Fusion Systems (CFS) and researchers from MIT’s Plasma Science and Fusion Center. While the calculation required an extraordinary amount of computer time, over 8 million CPU-hours, what was remarkable was not how much time was used, but how little, given the daunting computational challenge.

      The computational challenge of fusion energyTurbulence, which is the mechanism for most of the heat loss in a confined plasma, is one of the science’s grand challenges and the greatest problem remaining in classical physics. The equations that govern fusion plasmas are well known, but analytic solutions are not possible in the regimes of interest, where nonlinearities are important and solutions encompass an enormous range of spatial and temporal scales. Scientists resort to solving the equations by numerical simulation on computers. It is no accident that fusion researchers have been pioneers in computational physics for the last 50 years.

      One of the fundamental problems for researchers is reliably predicting plasma temperature and density given only the magnetic field configuration and the externally applied input power. In confinement devices like SPARC, the external power and the heat input from the fusion process are lost through turbulence in the plasma. The turbulence itself is driven by the difference in the extremely high temperature of the plasma core and the relatively cool temperatures of the plasma edge (merely a few million degrees). Predicting the performance of a self-heated fusion plasma therefore requires a calculation of the power balance between the fusion power input and the losses due to turbulence.

      These calculations generally start by assuming plasma temperature and density profiles at a particular location, then computing the heat transported locally by turbulence. However, a useful prediction requires a self-consistent calculation of the profiles across the entire plasma, which includes both the heat input and turbulent losses. Directly solving this problem is beyond the capabilities of any existing computer, so researchers have developed an approach that stitches the profiles together from a series of demanding but tractable local calculations. This method works, but since the heat and particle fluxes depend on multiple parameters, the calculations can be very slow to converge.

      However, techniques emerging from the field of machine learning are well suited to optimize just such a calculation. Starting with a set of computationally intensive local calculations run with the full-physics, first-principles CGYRO code (provided by a team from General Atomics led by Jeff Candy) Rodriguez-Fernandez and Howard fit a surrogate mathematical model, which was used to explore and optimize a search within the parameter space. The results of the optimization were compared to the exact calculations at each optimum point, and the system was iterated to a desired level of accuracy. The researchers estimate that the technique reduced the number of runs of the CGYRO code by a factor of four.

      New approach increases confidence in predictionsThis work, described in a recent publication in the journal Nuclear Fusion, is the highest fidelity calculation ever made of the core of a fusion plasma. It refines and confirms predictions made with less demanding models. Professor Jonathan Citrin, of the Eindhoven University of Technology and leader of the fusion modeling group for DIFFER, the Dutch Institute for Fundamental Energy Research, commented: “The work significantly accelerates our capabilities in more routinely performing ultra-high-fidelity tokamak scenario prediction. This algorithm can help provide the ultimate validation test of machine design or scenario optimization carried out with faster, more reduced modeling, greatly increasing our confidence in the outcomes.” 

      In addition to increasing confidence in the fusion performance of the SPARC experiment, this technique provides a roadmap to check and calibrate reduced physics models, which run with a small fraction of the computational power. Such models, cross-checked against the results generated from turbulence simulations, will provide a reliable prediction before each SPARC discharge, helping to guide experimental campaigns and improving the scientific exploitation of the device. It can also be used to tweak and improve even simple data-driven models, which run extremely quickly, allowing researchers to sift through enormous parameter ranges to narrow down possible experiments or possible future machines.

      The research was funded by CFS, with computational support from the National Energy Research Scientific Computing Center, a U.S. Department of Energy Office of Science User Facility. More

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      Using excess heat to improve electrolyzers and fuel cells

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      Reducing the use of fossil fuels will have unintended consequences for the power-generation industry and beyond. For example, many industrial chemical processes use fossil-fuel byproducts as precursors to things like asphalt, glycerine, and other important chemicals. One solution to reduce the impact of the loss of fossil fuels on industrial chemical processes is to store and use the heat that nuclear fission produces. New MIT research has dramatically improved a way to put that heat toward generating chemicals through a process called electrolysis. 

      Electrolyzers are devices that use electricity to split water (H2O) and generate molecules of hydrogen (H2) and oxygen (O2). Hydrogen is used in fuel cells to generate electricity and drive electric cars or drones or in industrial operations like the production of steel, ammonia, and polymers. Electrolyzers can also take in water and carbon dioxide (CO2) and produce oxygen and ethylene (C2H4), a chemical used in polymers and elsewhere.

      There are three main types of electrolyzers. One type works at room temperature, but has downsides; they’re inefficient and require rare metals, such as platinum. A second type is more efficient but runs at high temperatures, above 700 degrees Celsius. But metals corrode at that temperature, and the devices need expensive sealing and insulation. The third type would be a Goldilocks solution for nuclear heat if it were perfected, running at 300-600 C and requiring mostly cheap materials like stainless steel. These cells have never been operated as efficiently as theory says they should. The new work, published this month in Nature, both illuminates the problem and offers a solution.

      A sandwich mystery

      The intermediate-temperature devices use what are called protonic ceramic electrochemical cells. Each cell is a sandwich, with a dense electrolyte layered between two porous electrodes. Water vapor is pumped into the top electrode. A wire on the side connects the two electrodes, and externally generated electricity runs from the top to the bottom. The voltage pulls electrons out of the water, which splits the molecule, releasing oxygen. A hydrogen atom without an electron is just a proton. The protons get pulled through the electrolyte to rejoin with the electrons at the bottom electrode and form H2 molecules, which are then collected.

      On its own, the electrolyte in the middle, made mainly of barium, cerium, and zirconium, conducts protons very well. “But when we put the same material into this three-layer device, the proton conductivity of the full cell is pretty bad,” says Yanhao Dong, a postdoc in MIT’s Department of Nuclear Science and Engineering and a paper co-author. “Its conductivity is only about 50 percent of the bulk form’s. We wondered why there’s an inconsistency here.”

      A couple of clues pointed them in the right direction. First, if they don’t prepare the cell very carefully, the top layer, only about 20 microns (.02 millimeters) thick, doesn’t stay attached. “Sometimes if you use just Scotch tape, it will peel off,” Dong says. Second, when they looked at a cross section of a device using a scanning electron microscope, they saw that the top surface of the electrolyte layer was flat, whereas the bottom surface of the porous electrode sitting on it was bumpy, and the two came into contact in only a few places. They didn’t bond well. That precarious interface leads to both structural de-lamination and poor proton passage from the electrode to the electrolyte.

      Acidic solution

      The solution turned out to be simple: researchers roughed up the top of the electrolyte. Specifically, they applied acid for 10 minutes, which etched grooves into the surface. Ju Li, the Battelle Energy Alliance Professor in Nuclear Engineering and professor of materials science and engineering at MIT, and a paper co-author, likens it to sandblasting a surface before applying paint to increase adhesion. Their acid-treated cells produced about 200 percent more hydrogen per area at 1.5 volts at 600 C than did any previous cell of its type, and worked well down to 350 C with very little performance decay over extended operation. 

      “The authors reported a surprisingly simple yet highly effective surface treatment to dramatically improve the interface,” says Liangbing Hu, the director of the Center for Materials Innovation at the Maryland Energy Innovation Institute, who was not involved in the work. He calls the cell performance “exceptional.”

      “We are excited and surprised” by the results, Dong says. “The engineering solution seems quite simple. And that’s actually good, because it makes it very applicable to real applications.” In a practical product, many such cells would be stacked together to form a module. MIT’s partner in the project, Idaho National Laboratory, is very strong in engineering and prototyping, so Li expects to see electrolyzers based on this technology at scale before too long. “At the materials level, this is a breakthrough that shows that at a real-device scale you can work at this sweet spot of temperature of 350 to 600 degrees Celsius for nuclear fission and fusion reactors,” he says.

      “Reduced operating temperature enables cheaper materials for the large-scale assembly, including the stack,” says Idaho National Laboratory researcher and paper co-author Dong Ding. “The technology operates within the same temperature range as several important, current industrial processes, including ammonia production and CO2 reduction. Matching these temperatures will expedite the technology’s adoption within the existing industry.”

      “This is very significant for both Idaho National Lab and us,” Li adds, “because it bridges nuclear energy and renewable electricity.” He notes that the technology could also help fuel cells, which are basically electrolyzers run in reverse, using green hydrogen or hydrocarbons to generate electricity. According to Wei Wu, a materials scientist at Idaho National Laboratory and a paper co-author, “this technique is quite universal and compatible with other solid electrochemical devices.”

      Dong says it’s rare for a paper to advance both science and engineering to such a degree. “We are happy to combine those together and get both very good scientific understanding and also very good real-world performance.”

      This work, done in collaboration with Idaho National Laboratory, New Mexico State University, and the University of Nebraska–Lincoln, was funded, in part, by the U.S. Department of Energy. More

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      in Energy

      Finding the questions that guide MIT fusion research

      by

      “One of the things I learned was, doing good science isn’t so much about finding the answers as figuring out what the important questions are.”

      As Martin Greenwald retires from the responsibilities of senior scientist and deputy director of the MIT Plasma Science and Fusion Center (PSFC), he reflects on his almost 50 years of science study, 43 of them as a researcher at MIT, pursuing the question of how to make the carbon-free energy of fusion a reality.

      Most of Greenwald’s important questions about fusion began after graduating from MIT with a BS in both physics and chemistry. Beginning graduate work at the University of California at Berkeley, he felt compelled to learn more about fusion as an energy source that could have “a real societal impact.” At the time, researchers were exploring new ideas for devices that could create and confine fusion plasmas. Greenwald worked on Berkeley’s “alternate concept” TORMAC, a Toroidal Magnetic Cusp. “It didn’t work out very well,” he laughs. “The first thing I was known for was making the measurements that shut down the program.”

      Believing the temperature of the plasma generated by the device would not be as high as his group leader expected, Greenwald developed hardware that could measure the low temperatures predicted by his own “back of the envelope calculations.” As he anticipated, his measurements showed that “this was not a fusion plasma; this was hardly a confined plasma at all.”

      With a PhD from Berkeley, Greenwald returned to MIT for a research position at the PSFC, attracted by the center’s “esprit de corps.”

      He arrived in time to participate in the final experiments on Alcator A, the first in a series of tokamaks built at MIT, all characterized by compact size and featuring high-field magnets. The tokamak design was then becoming favored as the most effective route to fusion: its doughnut-shaped vacuum chamber, surrounded by electromagnets, could confine the turbulent plasma long enough, while increasing its heat and density, to make fusion occur.

      Alcator A showed that the energy confinement time improves in relation to increasing plasma density. MIT’s succeeding device, Alcator C, was designed to use higher magnetic fields, boosting expectations that it would reach higher densities and better confinement. To attain these goals, however, Greenwald had to pursue a new technique that increased density by injecting pellets of frozen fuel into the plasma, a method he likens to throwing “snowballs in hell.” This work was notable for the creation of a new regime of enhanced plasma confinement on Alcator C. In those experiments, a confined plasma surpassed for the first time one of the two Lawson criteria — the minimum required value for the product of the plasma density and confinement time — for making net power from fusion. This had been a milestone for fusion research since their publication by John Lawson in 1957.

      Greenwald continued to make a name for himself as part of a larger study into the physics of the Compact Ignition Tokamak — a high-field burning plasma experiment that the U.S. program was proposing to build in the late 1980s. The result, unexpectedly, was a new scaling law, later known as the “Greenwald Density Limit,” and a new theory for the mechanism of the limit. It has been used to accurately predict performance on much larger machines built since.

      The center’s next tokamak, Alcator C-Mod, started operation in 1993 and ran for more than 20 years, with Greenwald as the chair of its Experimental Program Committee. Larger than Alcator C, the new device supported a highly shaped plasma, strong radiofrequency heating, and an all-metal plasma-facing first wall. All of these would eventually be required in a fusion power system.

      C-Mod proved to be MIT’s most enduring fusion experiment to date, producing important results for 20 years. During that time Greenwald contributed not only to the experiments, but to mentoring the next generation. Research scientist Ryan Sweeney notes that “Martin quickly gained my trust as a mentor, in part due to his often casual dress and slightly untamed hair, which are embodiments of his transparency and his focus on what matters. He can quiet a room of PhDs and demand attention not by intimidation, but rather by his calmness and his ability to bring clarity to complicated problems, be they scientific or human in nature.”

      Greenwald worked closely with the group of students who, in PSFC Director Dennis Whyte’s class, came up with the tokamak concept that evolved into SPARC. MIT is now pursuing this compact, high-field tokamak with Commonwealth Fusion Systems, a startup that grew out of the collective enthusiasm for this concept, and the growing realization it could work. Greenwald now heads the Physics Group for the SPARC project at MIT. He has helped confirm the device’s physics basis in order to predict performance and guide engineering decisions.

      “Martin’s multifaceted talents are thoroughly embodied by, and imprinted on, SPARC” says Whyte. “First, his leadership in its plasma confinement physics validation and publication place SPARC on a firm scientific footing. Secondly, the impact of the density limit he discovered, which shows that fuel density increases with magnetic field and decreasing the size of the tokamak, is critical in obtaining high fusion power density not just in SPARC, but in future power plants. Third, and perhaps most impressive, is Martin’s mentorship of the SPARC generation of leadership.”

      Greenwald’s expertise and easygoing personality have made him an asset as head of the PSFC Office for Computer Services and group leader for data acquisition and computing, and sought for many professional committees. He has been an APS Fellow since 2000, and was an APS Distinguished Lecturer in Plasma Physics (2001-02). He was also presented in 2014 with a Leadership Award from Fusion Power Associates. He is currently an associate editor for Physics of Plasmas and a member of the Lawrence Livermore National Laboratory Physical Sciences Directorate External Review Committee.

      Although leaving his full-time responsibilities, Greenwald will remain at MIT as a visiting scientist, a role he says will allow him to “stick my nose into everything without being responsible for anything.”

      “At some point in the race you have to hand off the baton,“ he says. “And it doesn’t mean you’re not interested in the outcome; and it doesn’t mean you’re just going to walk away into the stands. I want to be there at the end when we succeed.” More