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      in Security

      A new way to swiftly eliminate micropollutants from water

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      “Zwitterionic” might not be a word you come across every day, but for Professor Patrick Doyle of the MIT Department of Chemical Engineering, it’s a word that’s central to the technology his group is developing to remove micropollutants from water. Derived from the German word “zwitter,” meaning “hybrid,” “zwitterionic” molecules are those with an equal number of positive and negative charges.

      Devashish Gokhale, a PhD student in Doyle’s lab, uses the example of a magnet to describe zwitterionic materials. “On a magnet, you have a north pole and a south pole that stick to each other, and on a zwitterionic molecule, you have a positive charge and a negative charge which stick to each other in a similar way.” Because many inorganic micropollutants and some organic micropollutants are themselves charged, Doyle and his team have been investigating how to deploy zwitterionic molecules to capture micropollutants in water. 

      In a new paper in Nature Water, Doyle, Gokhale, and undergraduate student Andre Hamelberg explain how they use zwitterionic hydrogels to sustainably capture both organic and inorganic micropollutants from water with minimal operational complexity. In the past, zwitterionic molecules have been used as coatings on membranes for water treatment because of their non-fouling properties. But in the Doyle group’s system, zwitterionic molecules are used to form the scaffold material, or backbone within the hydrogel — a porous three-dimensional network of polymer chains that contains a significant amount of water. “Zwitterionic molecules have very strong attraction to water compared to other materials which are used to make hydrogels or polymers,” says Gokhale. What’s more, the positive and negative charges on zwitterionic molecules cause the hydrogels to have lower compressibility than what has been commonly observed in hydrogels. This makes for significantly more swollen, robust, and porous hydrogels, which is important for the scale up of the hydrogel-based system for water treatment.

      The early stages of this research were supported by a seed grant from MIT’s Abdul Latif Jameel Water and Food Systems Lab (J-WAFS). Doyle’s group is now pursuing commercialization of the platform for both at-home use and industrial scale applications, with support from a J-WAFS Solutions grant.

      Seeking a sustainable solution

      Micropollutants are chemically diverse materials that can be harmful to human health and the environment, even though they are typically found at low concentrations (micrograms to milligrams per liter) relative to conventional contaminants. Micropollutants can be organic or inorganic and can be naturally-occurring or synthetic. Organic micropollutants are mostly carbon-based molecules and include pesticides and per- and polyfluoroalkyl substances (PFAS), known as “forever chemicals.” Inorganic micropollutants, such as heavy metals like lead and arsenic, tend to be smaller than organic micropollutants. Unfortunately, both organic and inorganic micropollutants are pervasive in the environment.

      Many micropollutants come from industrial processes, but the effects of human-induced climate change are also contributing to the environmental spread of micropollutants. Gokhale explains that, in California, for example, fires burn plastic electrical cables and leech micropollutants into natural ecosystems. Doyle adds that “outside of climate change, things like pandemics can spike the number of organic micropollutants in the environment due to high concentrations of pharmaceuticals in wastewater.”

      It’s no surprise then, that over the past few years micropollutants have become more and more of a concern. These chemicals have garnered attention in the media and led to “significant change in the environmental engineering and regulatory landscape” says Gokhale. In March 2023, the U.S. Environmental Protection Agency (EPA) proposed a strict, federal standard that would regulate six different PFAS chemicals in drinking water. Just last October, the EPA proposed banning the micropollutant trichloroethylene, a cancer-causing chemical that can be found in brake cleaners and other consumer products. And as recently as November, the EPA proposed that water utilities nationwide be required to replace all of their lead pipes to protect the public from lead exposure. Internationally, Gokhale notes the Oslo Paris Convention, whose mission is to protect the marine environment of the northeast Atlantic Ocean, including phasing out the discharge of offshore chemicals from the oil and gas industries. 

      With each new, necessary regulation to protect the safety of our water resources, the need for effective water treatment processes grows. Compounding this challenge is the need to make water treatment processes that are sustainable and energy-efficient. 

      The benchmark method to treat micropollutants in water is activated carbon. However, making filters with activated carbon is energy-intensive, requiring very high temperatures in large, centralized facilities. Gokhale says approximately “four kilograms of coal are needed to make one kilogram of activated carbon, so you lose a significant amount of carbon dioxide to the environment.” According to the World Economic Forum, global water and wastewater treatment accounts for 5 percent of annual emissions. In the U.S. alone, the EPA reports that drinking water and wastewater systems account for over 45 million tons of greenhouse gas emissions annually.

      “We need to develop methods which have smaller climate footprints than methods which are being used industrially today,” says Gokhale.

      Supporting a “high-risk” project

      In September 2019, Doyle and his lab embarked on an initial project to develop a microparticle-based platform to remove a broad range of micropollutants from water. Doyle’s group had been using hydrogels in pharmaceutical processing to formulate drug molecules into pill format. When he learned about the J-WAFS seed grant opportunity for early-stage research in water and food systems, Doyle realized his pharmaceutical work with hydrogels could be applied to environmental issues like water treatment. “I would never have gotten funding for this project if I went to the NSF [National Science Foundation], because they would just say, ‘you’re not a water person.’ But the J-WAFS seed grant offered a way for a high-risk, high-reward kind of project,” Doyle says.

      In March 2022, Doyle, Gokhale, and MIT undergraduate Ian Chen published findings from the seed grant work, describing their use of micelles within hydrogels for water treatment. Micelles are spherical structures that form when molecules called surfactants (found in things like soap), come in contact with water or other liquids. The team was able to synthesize micelle-laden hydrogel particles that soak up micropollutants from water like a sponge. Unlike activated carbon, the hydrogel particle system is made from environmentally friendly materials. Furthermore, the system’s materials are made at room temperature, making them exceedingly more sustainable than activated carbon.

      Building off the success of the seed grant, Doyle and his team were awarded a J-WAFS Solutions grant in September 2022 to help move their technology from the lab to the market. With this support, the researchers have been able to build, test, and refine pilot-scale prototypes of their hydrogel platform. System iterations during the solutions grant period have included the use of the zwitterionic molecules, a novel advancement from the seed grant work.  

      Rapid elimination of micropollutants is of special importance in commercial water treatment processes, where there is a limited amount of time water can spend inside the operational filtration unit. This is referred to as contact time, explains Gokhale. In municipal-scale or industrial-scale water treatment systems, contact times are usually less than 20 minutes and can be as short as five minutes. 

      “But as people have been trying to target these emerging micropollutants of concern, they realized they can’t get to sufficiently low concentrations on the same time scales as conventional contaminants,” Gokhale says. “Most technologies focus only on specific molecules or specific classes of molecules. So, you have whole technologies which are focusing only on PFAS, and then you have other technologies for lead and metals. When you start thinking about removing all of these contaminants from water, you end up with designs which have a very large number of unit operations. And that’s an issue because you have plants which are in the middle of large cities, and they don’t necessarily have space to expand to increase their contact times to efficiently remove multiple micropollutants,” he adds.

      Since zwitterionic molecules possess unique properties that confer high porosity, the researchers have been able to engineer a system for quicker uptake of micropollutants from water. Tests show that the hydrogels can eliminate six chemically diverse micropollutants at least 10 times faster than commercial activated carbon. The system is also compatible with a diverse set of materials, making it multifunctional. Micropollutants can bind to many different sites within the hydrogel platform: organic micropollutants bind to the micelles or surfactants while inorganic micropollutants bind to the zwitterionic molecules. Micelles, surfactants, zwitterionic molecules, and other chelating agents can be swapped in and out to essentially tune the system with different functionalities based on the profile of the water being treated. This kind of “plug-and-play” addition of various functional agents does not require a change in the design or synthesis of the hydrogel platform, and adding more functionalities does not take away from existing functionality. In this way, the zwitterionic-based system can rapidly remove multiple contaminants at lower concentrations in a single step, without the need for large, industrial units or capital expenditure. 

      Perhaps most importantly, the particles in the Doyle group’s system can be regenerated and used over and over again. By simply soaking the particles in an ethanol bath, they can be washed of micropollutants for indefinite use without loss of efficacy. When activated carbon is used for water treatment, the activated carbon itself becomes contaminated with micropollutants and must be treated as toxic chemical waste and disposed of in special landfills. Over time, micropollutants in landfills will reenter the ecosystem, perpetuating the problem.

      Arjav Shah, a PhD-MBA candidate in MIT’s Department of Chemical Engineering and the MIT Sloan School of Management, respectively, recently joined the team to lead commercialization efforts. The team has found that the zwitterionic hydrogels could be used in several real-world contexts, ranging from large-scale industrial packed beds to small-scale, portable, off-grid applications — for example, in tablets that could clean water in a canteen — and they have begun piloting the technology through a number of commercialization programs at MIT and in the greater Boston area.

      The combined strengths of each member of the team continue to drive the project forward in impactful ways, including undergraduate students like Andre Hamelberg, the third author on the Nature Water paper. Hamelberg is a participant in MIT’s Undergraduate Research Opportunities Program (UROP). Gokhale, who is also a J-WAFS Fellow, provides training and mentorship to Hamelberg and other UROP students in the lab.

      “We see this as an educational opportunity,” says Gokhale, noting that the UROP students learn science and chemical engineering through the research they conduct in the lab. The J-WAFS project has also been “a way of getting undergrads interested in water treatment and the more sustainable aspects of chemical engineering,” Gokhale says. He adds that it’s “one of the few projects which goes all the way from designing specific chemistries to building small filters and units and scaling them up and commercializing them. It’s a really good learning opportunity for the undergrads and we’re always excited to have them work with us.”

      In four years, the technology has been able to grow from an initial idea to a technology with scalable, real-world applications, making it an exemplar J-WAFS project. The fruitful collaboration between J-WAFS and the Doyle lab serves as inspiration for any MIT faculty who may want to apply their research to water or food systems projects.

      “The J-WAFS project serves as a way to demystify what a chemical engineer does,” says Doyle. “I think that there’s an old idea of chemical engineering as working in just oil and gas. But modern chemical engineering is focused on things which make life and the environment better.” More

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      in Environment

      MIT campus goals in food, water, waste support decarbonization efforts

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      With the launch of Fast Forward: MIT’s Climate Action Plan for the Decade, the Institute committed to decarbonize campus operations by 2050 — an effort that touches on every corner of MIT, from building energy use to procurement and waste. At the operational level, the plan called for establishing a set of quantitative climate impact goals in the areas of food, water, and waste to inform the campus decarbonization roadmap. After an 18-month process that engaged staff, faculty, and researchers, the goals — as well as high-level strategies to reach them — were finalized in spring 2023.

      The goal development process was managed by a team representing the areas of campus food, water, and waste, respectively, and includes Director of Campus Dining Mark Hayes and Senior Sustainability Project Manager Susy Jones (food), Director of Utilities Janine Helwig (water), Assistant Director of Campus Services Marty O’Brien, and Assistant Director of Sustainability Brain Goldberg (waste) to co-lead the efforts. The group worked together to set goals that leverage ongoing campus sustainability efforts. “It was important for us to collaborate in order to identify the strategies and goals,” explains Goldberg. “It allowed us to set goals that not only align, but build off of one another, enabling us to work more strategically.”

      In setting the goals, each team relied on data, community insight, and best practices. The co-leads are sharing their process to help others at the Institute understand the roles they can play in supporting these objectives.  

      Sustainable food systems

      The primary food impact goal aims for a 25 percent overall reduction in the greenhouse gas footprint of food purchases starting with academic year 2021-22 as a baseline, acknowledging that beef purchases make up a significant share of those emissions. Additionally, the co-leads established a goal to recover all edible food waste in dining hall and retail operations where feasible, as that reduces MIT’s waste impact and acknowledges that redistributing surplus food to feed people is critically important.

      The work to develop the food goal was uniquely challenging, as MIT works with nine different vendors — including main vendor Bon Appetit — to provide food on campus, with many vendors having their own sustainability targets. The goal-setting process began by understanding vendor strategies and leveraging their climate commitments. “A lot of this work is not about reinventing the wheel, but about gathering data,” says Hayes. “We are trying to connect the dots of what is currently happening on campus and to better understand food consumption and waste, ensuring that we area reaching these targets.”

      In identifying ways to reach and exceed these targets, Jones conducted listening sessions around campus, balancing input with industry trends, best-available science, and institutional insight from Hayes. “Before we set these goals and possible strategies, we wanted to get a grounding from the community and understand what would work on our campus,” says Jones, who recently began a joint role that bridges the Office of Sustainability and MIT Dining in part to support the goal work.

      By establishing the 25 percent reduction in the greenhouse gas footprint of food purchases across MIT residential dining menus, Jones and Hayes saw goal-setting as an opportunity to add more sustainable, local, and culturally diverse foods to the menu. “If beef is the most carbon-intensive food on the menu, this enables us to explore and expand so many recipes and menus from around the globe that incorporate alternatives,” Jones says.

      Strategies to reach the climate food goals focus on local suppliers, more plant-forward meals, food recovery, and food security. In 2019, MIT was a co-recipient of the New England Food Vision Prize provided by the Kendall Foundation to increase the amount of local food served on campus in partnership with CommonWealth Kitchen in Dorchester. While implementation of that program was put on pause due to the pandemic, work resumed this year. Currently, the prize is funding a collaborative effort to introduce falafel-like, locally manufactured fritters made from Maine-grown yellow field peas to dining halls at MIT and other university campuses, exemplifying the efforts to meet the climate impact goal, serve as a model for others, and provide demonstrable ways of strengthening the regional food system.

      “This sort of innovation is where we’re a leader,” says Hayes. “In addition to the Kendall Prize, we are looking to focus on food justice, growing our BIPOC [Black, Indigenous, and people of color] vendors, and exploring ideas such as local hydroponic and container vegetable growing companies, and how to scale these types of products into institutional settings.”

      Reduce and reuse for campus water

      The 2030 water impact goal aims to achieve a 10 percent reduction in water use compared to the 2019 baseline and to update the water reduction goal to align with the new metering program and proposed campus decarbonization plans as they evolve.

      When people think of campus water use, they may think of sprinklers, lab sinks, or personal use like drinking water and showers. And while those uses make up around 60 percent of campus water use, the Central Utilities Plant (CUP) accounts for the remaining 40 percent. “The CUP generates electricity and delivers heating and cooling to the campus through steam and chilled water — all using what amounts to a large percentage of water use on campus,” says Helwig. As such, the water goal focuses as much on reuse as reduction, with one approach being to expand water capture from campus cooling towers for reuse in CUP operations. “People often think of water use and energy separately, but they often go hand-in-hand,” Helwig explains.

      Data also play a central part in the water impact goal — that’s why a new metering program is called for in the implementation strategy. “We have access to a lot of data at MIT, but in reviewing the water data to inform the goal, we learned that it wasn’t quite where we needed it,” explains Helwig. “By ensuring we have the right meter and submeters set up, we can better set boundaries to understand where there is the potential to reduce water use.” Irrigation on campus is one such target with plans to soon release new campuswide landscaping standards that minimize water use.

      Reducing campus waste

      The waste impact goal aims to reduce campus trash by 30 percent compared to 2019 baseline totals. Additionally, the goal outlines efforts to improve the accuracy of indicators tracking campus waste; reduce the percentage of food scraps in trash and percent of recycling in trash in select locations; reduce the percentage of trash and recycling comprised of single use items; and increase the percentage of residence halls and other campus spaces where food is consumed at scale, implementing an MIT food scrap collection program.

      In setting the waste goals, Goldberg and O’Brien studied available campus waste data from past waste audits, pilot programs, and MIT’s waste haulers. They factored in state and city policies that regulate things like the type and amount of waste large institutions can transport. “Looking at all the data it became clear that a 30 percent trash reduction goal will make a tremendous impact on campus and help us drive toward the goal of completely designing out waste from campus,” Goldberg says. The strategies to reach the goals include reducing the amount of materials that come into campus, increasing recycling rates, and expanding food waste collection on campus.

      While reducing the waste created from material sources is outlined in the goals, food waste is a special focus on campus because it comprises approximately 40 percent of campus trash, it can be easily collected separately from trash and recycled locally, and decomposing food waste is one of the largest sources of greenhouse gas emissions found in landfills. “There is a lot of greenhouse gas emissions that result from production, distribution, transportation, packaging, processing, and disposal of food,” explains Goldberg. “When food travels to campus, is removed from campus as waste, and then breaks down in a landfill, there are emissions every step of the way.”

      To reduce food waste, Goldberg and O’Brien outlined strategies that include working with campus suppliers to identify ordering volumes and practices to limit waste. Once materials are on campus, another strategy kicks in, with a new third stream of waste collection that joins recycling and trash — food waste. By collecting the food waste separately — in bins that are currently rolling out across campus — the waste can be reprocessed into fertilizer, compost, and/or energy without the off-product of greenhouse gases. The waste impact goal also relies on behavioral changes to reduce waste, with education materials part of the process to reduce waste and decontaminate reprocessing streams.

      Tracking progress

      As work toward the goals advances, community members can monitor progress in the Sustainability DataPool Material Matters and Campus Water Use dashboards, or explore the Impact Goals in depth.

      “From food to water to waste, everyone on campus interacts with these systems and can grapple with their impact either from a material they need to dispose of, to water they’re using in a lab, or leftover food from an event,” says Goldberg. “By setting these goals we as an institution can lead the way and help our campus community understand how they can play a role, plug in, and make an impact.” More

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      in Energy

      Accelerated climate action needed to sharply reduce current risks to life and life-support systems

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      Hottest day on record. Hottest month on record. Extreme marine heatwaves. Record-low Antarctic sea-ice.

      While El Niño is a short-term factor in this year’s record-breaking heat, human-caused climate change is the long-term driver. And as global warming edges closer to 1.5 degrees Celsius — the aspirational upper limit set in the Paris Agreement in 2015 — ushering in more intense and frequent heatwaves, floods, wildfires, and other climate extremes much sooner than many expected, current greenhouse gas emissions-reduction policies are far too weak to keep the planet from exceeding that threshold. In fact, on roughly one-third of days in 2023, the average global temperature was at least 1.5 C higher than pre-industrial levels. Faster and bolder action will be needed — from the in-progress United Nations Climate Change Conference (COP28) and beyond — to stabilize the climate and minimize risks to human (and nonhuman) lives and the life-support systems (e.g., food, water, shelter, and more) upon which they depend.

      Quantifying the risks posed by simply maintaining existing climate policies — and the benefits (i.e., avoided damages and costs) of accelerated climate action aligned with the 1.5 C goal — is the central task of the 2023 Global Change Outlook, recently released by the MIT Joint Program on the Science and Policy of Global Change.

      Based on a rigorous, integrated analysis of population and economic growth, technological change, Paris Agreement emissions-reduction pledges (Nationally Determined Contributions, or NDCs), geopolitical tensions, and other factors, the report presents the MIT Joint Program’s latest projections for the future of the earth’s energy, food, water, and climate systems, as well as prospects for achieving the Paris Agreement’s short- and long-term climate goals.

      The 2023 Global Change Outlook performs its risk-benefit analysis by focusing on two scenarios. The first, Current Trends, assumes that Paris Agreement NDCs are implemented through the year 2030, and maintained thereafter. While this scenario represents an unprecedented global commitment to limit greenhouse gas emissions, it neither stabilizes climate nor limits climate change. The second scenario, Accelerated Actions, extends from the Paris Agreement’s initial NDCs and aligns with its long-term goals. This scenario aims to limit and stabilize human-induced global climate warming to 1.5 C by the end of this century with at least a 50 percent probability. Uncertainty is quantified using 400-member ensembles of projections for each scenario.

      This year’s report also includes a visualization tool that enables a higher-resolution exploration of both scenarios.

      Energy

      Between 2020 and 2050, population and economic growth are projected to drive continued increases in energy needs and electrification. Successful achievement of current Paris Agreement pledges will reinforce a shift away from fossil fuels, but additional actions will be required to accelerate the energy transition needed to cap global warming at 1.5 C by 2100.

      During this 30-year period under the Current Trends scenario, the share of fossil fuels in the global energy mix drops from 80 percent to 70 percent. Variable renewable energy (wind and solar) is the fastest growing energy source with more than an 8.6-fold increase. In the Accelerated Actions scenario, the share of low-carbon energy sources grows from 20 percent to slightly more than 60 percent, a much faster growth rate than in the Current Trends scenario; wind and solar energy undergo more than a 13.3-fold increase.

      While the electric power sector is expected to successfully scale up (with electricity production increasing by 73 percent under Current Trends, and 87 percent under Accelerated Actions) to accommodate increased demand (particularly for variable renewables), other sectors face stiffer challenges in their efforts to decarbonize.

      “Due to a sizeable need for hydrocarbons in the form of liquid and gaseous fuels for sectors such as heavy-duty long-distance transport, high-temperature industrial heat, agriculture, and chemical production, hydrogen-based fuels and renewable natural gas remain attractive options, but the challenges related to their scaling opportunities and costs must be resolved,” says MIT Joint Program Deputy Director Sergey Paltsev, a lead author of the 2023 Global Change Outlook.

      Water, food, and land

      With a global population projected to reach 9.9 billion by 2050, the Current Trends scenario indicates that more than half of the world’s population will experience pressures to its water supply, and that three of every 10 people will live in water basins where compounding societal and environmental pressures on water resources will be experienced. Population projections under combined water stress in all scenarios reveal that the Accelerated Actions scenario can reduce approximately 40 million of the additional 570 million people living in water-stressed basins at mid-century.

      Under the Current Trends scenario, agriculture and food production will keep growing. This will increase pressure for land-use change, water use, and use of energy-intensive inputs, which will also lead to higher greenhouse gas emissions. Under the Accelerated Actions scenario, less agricultural and food output is observed by 2050 compared to the Current Trends scenario, since this scenario affects economic growth and increases production costs. Livestock production is more greenhouse gas emissions-intensive than crop and food production, which, under carbon-pricing policies, drives demand downward and increases costs and prices. Such impacts are transmitted to the food sector and imply lower consumption of livestock-based products.

      Land-use changes in the Accelerated Actions scenario are similar to those in the Current Trends scenario by 2050, except for land dedicated to bioenergy production. At the world level, the Accelerated Actions scenario requires cropland area to increase by 1 percent and pastureland to decrease by 4.2 percent, but land use for bioenergy must increase by 44 percent.

      Climate trends

      Under the Current Trends scenario, the world is likely (more than 50 percent probability) to exceed 2 C global climate warming by 2060, 2.8 C by 2100, and 3.8 C by 2150. Our latest climate-model information indicates that maximum temperatures will likely outpace mean temperature trends over much of North and South America, Europe, northern and southeast Asia, and southern parts of Africa and Australasia. So as human-forced climate warming intensifies, these regions are expected to experience more pronounced record-breaking extreme heat events.

      Under the Accelerated Actions scenario, global temperature will continue to rise through the next two decades. But by 2050, global temperature will stabilize, and then slightly decline through the latter half of the century.

      “By 2100, the Accelerated Actions scenario indicates that the world can be virtually assured of remaining below 2 C of global warming,” says MIT Joint Program Deputy Director C. Adam Schlosser, a lead author of the report. “Nevertheless, additional policy mechanisms must be designed with more comprehensive targets that also support a cleaner environment, sustainable resources, as well as improved and equitable human health.”

      The Accelerated Actions scenario not only stabilizes global precipitation increase (by 2060), but substantially reduces the magnitude and potential range of increases to almost one-third of Current Trends global precipitation changes. Any global increase in precipitation heightens flood risk worldwide, so policies aligned with the Accelerated Actions scenario would considerably reduce that risk.

      Prospects for meeting Paris Agreement climate goals

      Numerous countries and regions are progressing in fulfilling their Paris Agreement pledges. Many have declared more ambitious greenhouse gas emissions-mitigation goals, while financing to assist the least-developed countries in sustainable development is not forthcoming at the levels needed. In this year’s Global Stocktake Synthesis Report, the U.N. Framework Convention on Climate Change evaluated emissions reductions communicated by the parties of the Paris Agreement and concluded that global emissions are not on track to fulfill the most ambitious long-term global temperature goals of the Paris Agreement (to keep warming well below 2 C — and, ideally, 1.5 C — above pre-industrial levels), and there is a rapidly narrowing window to raise ambition and implement existing commitments in order to achieve those targets. The Current Trends scenario arrives at the same conclusion.

      The 2023 Global Change Outlook finds that both global temperature targets remain achievable, but require much deeper near-term emissions reductions than those embodied in current NDCs.

      Reducing climate risk

      This report explores two well-known sets of risks posed by climate change. Research highlighted indicates that elevated climate-related physical risks will continue to evolve by mid-century, along with heightened transition risks that arise from shifts in the political, technological, social, and economic landscapes that are likely to occur during the transition to a low-carbon economy.

      “Our Outlook shows that without aggressive actions the world will surpass critical greenhouse gas concentration thresholds and climate targets in the coming decades,” says MIT Joint Program Director Ronald Prinn. “While the costs of inaction are getting higher, the costs of action are more manageable.” More

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      in Environment

      In a surprising finding, light can make water evaporate without heat

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      Evaporation is happening all around us all the time, from the sweat cooling our bodies to the dew burning off in the morning sun. But science’s understanding of this ubiquitous process may have been missing a piece all this time.

      In recent years, some researchers have been puzzled upon finding that water in their experiments, which was held in a sponge-like material known as a hydrogel, was evaporating at a higher rate than could be explained by the amount of heat, or thermal energy, that the water was receiving. And the excess has been significant — a doubling, or even a tripling or more, of the theoretical maximum rate.

      After carrying out a series of new experiments and simulations, and reexamining some of the results from various groups that claimed to have exceeded the thermal limit, a team of researchers at MIT has reached a startling conclusion: Under certain conditions, at the interface where water meets air, light can directly bring about evaporation without the need for heat, and it actually does so even more efficiently than heat. In these experiments, the water was held in a hydrogel material, but the researchers suggest that the phenomenon may occur under other conditions as well.

      The findings are published this week in a paper in PNAS, by MIT postdoc Yaodong Tu, professor of mechanical engineering Gang Chen, and four others.

      The phenomenon might play a role in the formation and evolution of fog and clouds, and thus would be important to incorporate into climate models to improve their accuracy, the researchers say. And it might play an important part in many industrial processes such as solar-powered desalination of water, perhaps enabling alternatives to the step of converting sunlight to heat first.

      The new findings come as a surprise because water itself does not absorb light to any significant degree. That’s why you can see clearly through many feet of clean water to the surface below. So, when the team initially began exploring the process of solar evaporation for desalination, they first put particles of a black, light-absorbing material in a container of water to help convert the sunlight to heat.

      Then, the team came across the work of another group that had achieved an evaporation rate double the thermal limit — which is the highest possible amount of evaporation that can take place for a given input of heat, based on basic physical principles such as the conservation of energy. It was in these experiments that the water was bound up in a hydrogel. Although they were initially skeptical, Chen and Tu starting their own experiments with hydrogels, including a piece of the material from the other group. “We tested it under our solar simulator, and it worked,” confirming the unusually high evaporation rate, Chen says. “So, we believed them now.” Chen and Tu then began making and testing their own hydrogels.

      They began to suspect that the excess evaporation was being caused by the light itself —that photons of light were actually knocking bundles of water molecules loose from the water’s surface. This effect would only take place right at the boundary layer between water and air, at the surface of the hydrogel material — and perhaps also on the sea surface or the surfaces of droplets in clouds or fog.

      In the lab, they monitored the surface of a hydrogel, a JELL-O-like matrix consisting mostly of water bound by a sponge-like lattice of thin membranes. They measured its responses to simulated sunlight with precisely controlled wavelengths.

      The researchers subjected the water surface to different colors of light in sequence and measured the evaporation rate. They did this by placing a container of water-laden hydrogel on a scale and directly measuring the amount of mass lost to evaporation, as well as monitoring the temperature above the hydrogel surface. The lights were shielded to prevent them from introducing extra heat. The researchers found that the effect varied with color and peaked at a particular wavelength of green light. Such a color dependence has no relation to heat, and so supports the idea that it is the light itself that is causing at least some of the evaporation.

      The puffs of white condensation on glass is water being evaporated from a hydrogel using green light, without heat.Image: Courtesy of the researchers

      The researchers tried to duplicate the observed evaporation rate with the same setup but using electricity to heat the material, and no light. Even though the thermal input was the same as in the other test, the amount of water that evaporated never exceeded the thermal limit. However, it did so when the simulated sunlight was on, confirming that light was the cause of the extra evaporation.

      Though water itself does not absorb much light, and neither does the hydrogel material itself, when the two combine they become strong absorbers, Chen says. That allows the material to harness the energy of the solar photons efficiently and exceed the thermal limit, without the need for any dark dyes for absorption.

      Having discovered this effect, which they have dubbed the photomolecular effect, the researchers are now working on how to apply it to real-world needs. They have a grant from the Abdul Latif Jameel Water and Food Systems Lab to study the use of this phenomenon to improve the efficiency of solar-powered desalination systems, and a Bose Grant to explore the phenomenon’s effects on climate change modeling.

      Tu explains that in standard desalination processes, “it normally has two steps: First we evaporate the water into vapor, and then we need to condense the vapor to liquify it into fresh water.” With this discovery, he says, potentially “we can achieve high efficiency on the evaporation side.” The process also could turn out to have applications in processes that require drying a material.

      Chen says that in principle, he thinks it may be possible to increase the limit of water produced by solar desalination, which is currently 1.5 kilograms per square meter, by as much as three- or fourfold using this light-based approach. “This could potentially really lead to cheap desalination,” he says.

      Tu adds that this phenomenon could potentially also be leveraged in evaporative cooling processes, using the phase change to provide a highly efficient solar cooling system.

      Meanwhile, the researchers are also working closely with other groups who are attempting to replicate the findings, hoping to overcome skepticism that has faced the unexpected findings and the hypothesis being advanced to explain them.

      The research team also included Jiawei Zhou, Shaoting Lin, Mohammed Alshrah, and Xuanhe Zhao, all in MIT’s Department of Mechanical Engineering. More

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      in Environment

      Smart irrigation technology covers “more crop per drop”

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      In agriculture today, robots and drones can monitor fields, temperature and moisture sensors can be automated to meet crop needs, and a host of other systems and devices make farms more efficient, resource-conscious, and profitable. The use of precision agriculture, as these technologies are collectively known, offers significant advantages. However, because the technology can be costly, it remains out of reach for the majority of the world’s farmers.

      “Many of the poor around the world are small, subsistence farmers,” says Susan Amrose, research scientist with the Global Engineering and Research (GEAR) Lab at MIT. “With intensification of food production needs, worsening soil, water scarcity, and smaller plots, these farmers can’t continue with their current practices.”

      By some estimates, the global demand for fresh water will outstrip supply by as much as 40 percent by the end of the decade. Nearly 80 percent of the world’s 570 million farms are classed as smallholder farms, with many located in under-resourced and water-stressed regions. With rapid population growth and climate change driving up demand for food, and with more strain on natural resources, increasing the adoption of sustainable agricultural practices among smallholder farmers is vital. 

      Amrose, who helps lead desalination, drip irrigation, water, and sanitation projects for GEAR Lab, says these small farmers need to move to more mechanized practices. “We’re trying to make it much, much more affordable for farmers to utilize solar-powered irrigation, and to have access to tools that, right now, they’re priced out of,” she says. “More crop per drop, more crop per area, that’s our goal.”

      Play video

      No Drop to Spare: MIT creates affordable, user-driven smart irrigation technology | MIT Mechanical Engineering

      Drip irrigation systems release water and nutrients in controlled volumes directly to the root zone of the crop through a network of pipes and emitters. These systems can reduce water consumption by 20 to 60 percent when compared to conventional flood irrigation methods.

      “Agriculture uses 70 percent of the fresh water that’s in use across the globe. Large-scale adoption and correct management of drip irrigation could help to reduce consumption of fresh water, which is especially critical for regions experiencing water shortages or groundwater depletion,” says Carolyn Sheline SM ’19, a PhD student and member of the GEAR Lab’s Drip Irrigation team. “A lot of irrigation technology is developed for larger farms that can put more money into it — but inexpensive doesn’t need to mean ‘not technologically advanced.’”

      GEAR Lab has created several drip irrigation technology solutions to date, including a low-pressure drip emitter that has been shown to reduce pumping energy by more than 50 percent when compared to existing emitters; a systems-level optimization model that analyzes factors like local weather conditions and crop layouts, to cut overall system operation costs by up to 30 percent; and a low-cost precision irrigation controller that optimizes system energy and water use, enabling farmers to operate the system on an ideal schedule given their specific resources, needs, and preferences. The controller has recently been shown to reduce water consumption by over 40 percent when compared to traditional practices.

      To build these new, affordable technologies, the team tapped into a critical knowledge source — the farmers themselves.

      “We didn’t just create technology in isolation — we also advanced our understanding of how people would interact with and value this technology, and we did that before the technology had come to fruition,” says Amos Winter SM ’05, PhD ’11, associate professor of mechanical engineering and MIT GEAR Lab principal investigator. “Getting affirmations that farmers would value what the technology would do before we finished it was incredibly important.”

      The team held “Farmer Field Days” and conducted interviews with more than 200 farmers, suppliers, and industry professionals in Kenya, Morocco, and Jordan, the regions selected to host field pilot test sites. These specific sites were selected for a variety of reasons, including solar availability and water scarcity, and because all were great candidate markets for eventual adoption of the technology.

      “People usually understand their own problems really well, and they’re very good at coming up with solutions to them,” says Fiona Grant ’17, SM ’19, also a PhD candidate with the GEAR Lab Drip Irrigation team. “As designers, our role really is to provide a different set of expertise and another avenue for them to get the tools or the resources that they need.”

      The controller, for example, takes in weather information, like relative humidity, temperature, wind speed values, and precipitation. Then, using artificial intelligence, it calculates and predicts the area’s solar exposure for the day and the exact irrigation needs for the farmer, and sends information to their smartphone. How much, or how little, automation an individual site uses remains up to the farmer. In its first season of operation on a Moroccan test site, GEAR Lab technology reduced water consumption by 44 percent and energy by 38 percent when compared to a neighboring farm using traditional drip irrigation practice.

      “The way you’re going to operate a system is going to have a big impact on the way you design it,” says Grant. “We gained a sense of what farmers would be willing to change, or not, regarding interactions with the system. We found that what we might change, and what would be acceptable to change, were not necessarily the same thing.”

      GEAR Lab alumna Georgia Van de Zande ’15, SM ’18, PhD ’23, concurs. “It’s about more than just delivering a lower-cost system, it’s also about creating something they’re going to want to use and want to trust.”

      In Jordan, researchers at a full-scale test farm are operating a solar-powered drip system with a prototype of the controller and are receiving smartphone commands on when to open and close the manual valves. In Morocco, the controller is operating at a research farm with a fully automated hydraulic system; researchers are monitoring the irrigation and conducting additional agronomic tasks. In Kenya, where precision agriculture and smart irrigation haven’t yet seen very much adoption, a simpler version of the controller serves to provide educational and training information in addition to offering scheduling and control capabilities.

      Knowledge is power for the farmers, and for designers and engineers, too. If an engineer can know a user’s requirements, Winter says, they’re much more likely to create a successful solution.

      “The most powerful tool a designer can have is perspective. I have one perspective — the math and science and tech innovation side — but I don’t know a thing about what it’s like to live every day as a farmer in Jordan or Morocco,” says Winter. “I don’t know what clogs the filters, or who shuts off the water. If you can see the world through the eyes of stakeholders, you’re going to spot requirements and constraints that you wouldn’t have picked up on otherwise.”

      Winter says the technology his team is building is exciting for a lot of reasons.

      “To be in a situation where the world is saying, ‘we need to deal with water stress, we need to deal with climate adaptation, and we need to particularly do this in resource-constrained countries,’ and to be in a position where we can do something about it and produce something of tremendous value and efficacy is incredible,” says Winter. “Solving the right problem at the right time, on a massive scale, is thrilling.” More

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      in Energy

      Desalination system could produce freshwater that is cheaper than tap water

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      Engineers at MIT and in China are aiming to turn seawater into drinking water with a completely passive device that is inspired by the ocean, and powered by the sun.

      In a paper appearing today in the journal Joule, the team outlines the design for a new solar desalination system that takes in saltwater and heats it with natural sunlight.

      The configuration of the device allows water to circulate in swirling eddies, in a manner similar to the much larger “thermohaline” circulation of the ocean. This circulation, combined with the sun’s heat, drives water to evaporate, leaving salt behind. The resulting water vapor can then be condensed and collected as pure, drinkable water. In the meantime, the leftover salt continues to circulate through and out of the device, rather than accumulating and clogging the system.

      The new system has a higher water-production rate and a higher salt-rejection rate than all other passive solar desalination concepts currently being tested.

      The researchers estimate that if the system is scaled up to the size of a small suitcase, it could produce about 4 to 6 liters of drinking water per hour and last several years before requiring replacement parts. At this scale and performance, the system could produce drinking water at a rate and price that is cheaper than tap water.

      “For the first time, it is possible for water, produced by sunlight, to be even cheaper than tap water,” says Lenan Zhang, a research scientist in MIT’s Device Research Laboratory.

      The team envisions a scaled-up device could passively produce enough drinking water to meet the daily requirements of a small family. The system could also supply off-grid, coastal communities where seawater is easily accessible.

      Zhang’s study co-authors include MIT graduate student Yang Zhong and Evelyn Wang, the Ford Professor of Engineering, along with Jintong Gao, Jinfang You, Zhanyu Ye, Ruzhu Wang, and Zhenyuan Xu of Shanghai Jiao Tong University in China.

      A powerful convection

      The team’s new system improves on their previous design — a similar concept of multiple layers, called stages. Each stage contained an evaporator and a condenser that used heat from the sun to passively separate salt from incoming water. That design, which the team tested on the roof of an MIT building, efficiently converted the sun’s energy to evaporate water, which was then condensed into drinkable water. But the salt that was left over quickly accumulated as crystals that clogged the system after a few days. In a real-world setting, a user would have to place stages on a frequent basis, which would significantly increase the system’s overall cost.

      In a follow-up effort, they devised a solution with a similar layered configuration, this time with an added feature that helped to circulate the incoming water as well as any leftover salt. While this design prevented salt from settling and accumulating on the device, it desalinated water at a relatively low rate.

      In the latest iteration, the team believes it has landed on a design that achieves both a high water-production rate, and high salt rejection, meaning that the system can quickly and reliably produce drinking water for an extended period. The key to their new design is a combination of their two previous concepts: a multistage system of evaporators and condensers, that is also configured to boost the circulation of water — and salt — within each stage.

      “We introduce now an even more powerful convection, that is similar to what we typically see in the ocean, at kilometer-long scales,” Xu says.

      The small circulations generated in the team’s new system is similar to the “thermohaline” convection in the ocean — a phenomenon that drives the movement of water around the world, based on differences in sea temperature (“thermo”) and salinity (“haline”).

      “When seawater is exposed to air, sunlight drives water to evaporate. Once water leaves the surface, salt remains. And the higher the salt concentration, the denser the liquid, and this heavier water wants to flow downward,” Zhang explains. “By mimicking this kilometer-wide phenomena in small box, we can take advantage of this feature to reject salt.”

      Tapping out

      The heart of the team’s new design is a single stage that resembles a thin box, topped with a dark material that efficiently absorbs the heat of the sun. Inside, the box is separated into a top and bottom section. Water can flow through the top half, where the ceiling is lined with an evaporator layer that uses the sun’s heat to warm up and evaporate any water in direct contact. The water vapor is then funneled to the bottom half of the box, where a condensing layer air-cools the vapor into salt-free, drinkable liquid. The researchers set the entire box at a tilt within a larger, empty vessel, then attached a tube from the top half of the box down through the bottom of the vessel, and floated the vessel in saltwater.

      In this configuration, water can naturally push up through the tube and into the box, where the tilt of the box, combined with the thermal energy from the sun, induces the water to swirl as it flows through. The small eddies help to bring water in contact with the upper evaporating layer while keeping salt circulating, rather than settling and clogging.

      The team built several prototypes, with one, three, and 10 stages, and tested their performance in water of varying salinity, including natural seawater and water that was seven times saltier.

      From these tests, the researchers calculated that if each stage were scaled up to a square meter, it would produce up to 5 liters of drinking water per hour, and that the system could desalinate water without accumulating salt for several years. Given this extended lifetime, and the fact that the system is entirely passive, requiring no electricity to run, the team estimates that the overall cost of running the system would be cheaper than what it costs to produce tap water in the United States.

      “We show that this device is capable of achieving a long lifetime,” Zhong says. “That means that, for the first time, it is possible for drinking water produced by sunlight to be cheaper than tap water. This opens up the possibility for solar desalination to address real-world problems.”

      “This is a very innovative approach that effectively mitigates key challenges in the field of desalination,” says Guihua Yu, who develops sustainable water and energy storage systems at the University of Texas at Austin, and was not involved in the research. “The design is particularly beneficial for regions struggling with high-salinity water. Its modular design makes it highly suitable for household water production, allowing for scalability and adaptability to meet individual needs.”

      Funding for the research at Shanghai Jiao Tong University was supported by the Natural Science Foundation of China. More

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      in Environment

      Technologies for water conservation and treatment move closer to commercialization

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      The Abdul Latif Jameel Water and Food Systems Lab (J-WAFS) provides Solutions Grants to help MIT researchers launch startup companies or products to commercialize breakthrough technologies in water and food systems. The Solutions Grant Program began in 2015 and is supported by Community Jameel. In addition to one-year, renewable grants of up to $150,000, the program also matches grantees with industry mentors and facilitates introductions to potential investors. Since its inception, the J-WAFS Solutions Program has awarded over $3 million in funding to the MIT community. Numerous startups and products, including a portable desalination device and a company commercializing a novel food safety sensor, have spun out of this support.

      The 2023 J-WAFS Solutions Grantees are Professor C. Cem Tasan of the Department of Materials Science and Engineering and Professor Andrew Whittle of the Department of Civil and Environmental Engineering. Tasan’s project involves reducing water use in steel manufacturing and Whittle’s project tackles harmful algal blooms in water. Project work commences this September.

      “This year’s Solutions Grants are being award to professors Tasan and Whittle to help commercialize technologies they have been developing at MIT,” says J-WAFS executive director Renee J. Robins. “With J-WAFS’ support, we hope to see the teams move their technologies from the lab to the market, so they can have a beneficial impact on water use and water quality challenges,” Robins adds.

      Reducing water consumption by solid-state steelmaking

      Water is a major requirement for steel production. The steel industry ranks fourth in industrial freshwater consumption worldwide, since large amounts of water are needed mainly for cooling purposes in the process. Unfortunately, a strong correlation has also been shown to exist between freshwater use in steelmaking and water contamination. As the global demand for steel increases and freshwater availability decreases due to climate change, improved methods for more sustainable steel production are needed.

      A strategy to reduce the water footprint of steelmaking is to explore steel recycling processes that avoid liquid metal processing. With this motivation, Cem Tasan, the Thomas B. King Associate Professor of Metallurgy in the Department of Materials Science and Engineering, and postdoc Onur Guvenc PhD created a new process called Scrap Metal Consolidation (SMC). SMC is based on a well-established metal forming process known as roll bonding. Conventionally, roll bonding requires intensive prior surface treatment of the raw material, specific atmospheric conditions, and high deformation levels. Tasan and Guvenc’s research revealed that SMC can overcome these restrictions by enabling the solid-state bonding of scrap into a sheet metal form, even when the surface quality, atmospheric conditions, and deformation levels are suboptimal. Through lab-scale proof-of-principle investigations, they have already identified SMC process conditions and validated the mechanical formability of resulting steel sheets, focusing on mild steel, the most common sheet metal scrap.

      The J-WAFS Solutions Grant will help the team to build customer product prototypes, design the processing unit, and develop a scale-up strategy and business model. By simultaneously decreasing water usage, energy demand, contamination risk, and carbon dioxide burden, SMC has the potential to decrease the energy need for steel recycling by up to 86 percent, as well as reduce the linked carbon dioxide emissions and safeguard the freshwater resources that would otherwise be directed to industrial consumption. 

      Detecting harmful algal blooms in water before it’s too late

      Harmful algal blooms (HABs) are a growing problem in both freshwater and saltwater environments worldwide, causing an estimated $13 billion in annual damage to drinking water, water for recreational use, commercial fishing areas, and desalination activities. HABs pose a threat to both human health and aquaculture, thereby threatening the food supply. Toxins in HABs are produced by some cyanobacteria, or blue-green algae, whose communities change in composition in response to eutrophication from agricultural runoff, sewer overflows, or other events. Mitigation of risks from HABs are most effective when there is advance warning of these changes in algal communities. 

      Most in situ measurements of algae are based on fluorescence spectroscopy that is conducted with LED-induced fluorescence (LEDIF) devices, or probes that induce fluorescence of specific algal pigments using LED light sources. While LEDIFs provide reasonable estimates of concentrations of individual pigments, they lack resolution to discriminate algal classes within complex mixtures found in natural water bodies. In prior research, Andrew Whittle, the Edmund K. Turner Professor of Civil and Environmental Engineering, worked with colleagues to design REMORA, a low-cost, field-deployable prototype spectrofluorometer for measuring induced fluorescence. This research was part of a collaboration between MIT and the AMS Institute. Whittle and the team successfully trained a machine learning model to discriminate and quantify cell concentrations for mixtures of different algal groups in water samples through an extensive laboratory calibration program using various algae cultures. The group demonstrated these capabilities in a series of field measurements at locations in Boston and Amsterdam. 

      Whittle will work with Fábio Duarte of the Department of Urban Studies and Planning, the Senseable City Lab, and MIT’s Center for Real Estate to refine the design of REMORA. They will develop software for autonomous operation of the sensor that can be deployed remotely on mobile vessels or platforms to enable high-resolution spatiotemporal monitoring for harmful algae. Sensor commercialization will hopefully be able to exploit the unique capabilities of REMORA for long-term monitoring applications by water utilities, environmental regulatory agencies, and water-intensive industries.  More

    • 188 Shares189 Views

      in Environment

      New clean air and water labs to bring together researchers, policymakers to find climate solutions

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      MIT’s Abdul Latif Jameel Poverty Action Lab (J-PAL) is launching the Clean Air and Water Labs, with support from Community Jameel, to generate evidence-based solutions aimed at increasing access to clean air and water.

      Led by J-PAL’s Africa, Middle East and North Africa (MENA), and South Asia regional offices, the labs will partner with government agencies to bring together researchers and policymakers in areas where impactful clean air and water solutions are most urgently needed.

      Together, the labs aim to improve clean air and water access by informing the scaling of evidence-based policies and decisions of city, state, and national governments that serve nearly 260 million people combined.

      The Clean Air and Water Labs expand the work of J-PAL’s King Climate Action Initiative, building on the foundational support of King Philanthropies, which significantly expanded J-PAL’s work at the nexus of climate change and poverty alleviation worldwide. 

      Air pollution, water scarcity and the need for evidence 

      Africa, MENA, and South Asia are on the front lines of global air and water crises. 

      “There is no time to waste investing in solutions that do not achieve their desired effects,” says Iqbal Dhaliwal, global executive director of J-PAL. “By co-generating rigorous real-world evidence with researchers, policymakers can have the information they need to dedicate resources to scaling up solutions that have been shown to be effective.”

      In India, about 75 percent of households did not have drinking water on premises in 2018. In MENA, nearly 90 percent of children live in areas facing high or extreme water stress. Across Africa, almost 400 million people lack access to safe drinking water. 

      Simultaneously, air pollution is one of the greatest threats to human health globally. In India, extraordinary levels of air pollution are shortening the average life expectancy by five years. In Africa, rising indoor and ambient air pollution contributed to 1.1 million premature deaths in 2019. 

      There is increasing urgency to find high-impact and cost-effective solutions to the worsening threats to human health and resources caused by climate change. However, data and evidence on potential solutions are limited.

      Fostering collaboration to generate policy-relevant evidence 

      The Clean Air and Water Labs will foster deep collaboration between government stakeholders, J-PAL regional offices, and researchers in the J-PAL network. 

      Through the labs, J-PAL will work with policymakers to:

      co-diagnose the most pressing air and water challenges and opportunities for policy innovation;
      expand policymakers’ access to and use of high-quality air and water data;
      co-design potential solutions informed by existing evidence;
      co-generate evidence on promising solutions through rigorous evaluation, leveraging existing and new data sources; and
      support scaling of air and water policies and programs that are found to be effective through evaluation. 
      A research and scaling fund for each lab will prioritize resources for co-generated pilot studies, randomized evaluations, and scaling projects. 

      The labs will also collaborate with C40 Cities, a global network of mayors of the world’s leading cities that are united in action to confront the climate crisis, to share policy-relevant evidence and identify opportunities for potential new connections and research opportunities within India and across Africa.

      This model aims to strengthen the use of evidence in decision-making to ensure solutions are highly effective and to guide research to answer policymakers’ most urgent questions. J-PAL Africa, MENA, and South Asia’s strong on-the-ground presence will further bridge research and policy work by anchoring activities within local contexts. 

      “Communities across the world continue to face challenges in accessing clean air and water, a threat to human safety that has only been exacerbated by the climate crisis, along with rising temperatures and other hazards,” says George Richards, director of Community Jameel. “Through our collaboration with J-PAL and C40 in creating climate policy labs embedded in city, state, and national governments in Africa and South Asia, we are committed to innovative and science-based approaches that can help hundreds of millions of people enjoy healthier lives.”

      J-PAL Africa, MENA, and South Asia will formally launch Clean Air and Water Labs with government partners over the coming months. J-PAL is housed in the MIT Department of Economics, within the School of Humanities, Arts, and Social Sciences. More